Dielectric resonances in three-dimensional binary disordered media

Abstract:

Powdered solids often present very specific properties due to their granular nature. Such powders are often obtained by mixing two ingbkp_redients in variable proportions: conductor and insulator, or conductor and super-conductor. In a very natural way, these systems are modeled by regular lattices, whose sites or bonds are randomly chosen with given probabilities. It is known that the electrical and optical properties of random bi-dimensional (2D) networks are well described by their conductance's poles (resonances) and residues (amplitudes). The numerical implementation of a spectral method gave the spectral density, the AC conductivity, the multi-fractal properties of the moments for the local electric field (or currents), and spectrum of resonances characteristic of some small clusters (animals). This work extends the spectral method to the three-dimensional (3D) case where the problem is more complicated because the duality property and the corresponding symmetries are broken. As in the 2D-case, the two significant parameters are the ratio h = σ1/σ0 of the complex conductances σ0 and σ1 of both phases, and the probability p (resp. 1 - p) of σ0 (resp. σ1). All the resonances lie on the negative real h-axis, i.e. for pure non resistive networks in the AC case. For a static (DC) system, only the value h = 0 (corresponding to a binary system with σ0 finite and σ1 = 0, or σ0 = ∞ and σ1 finite) can give a resonance. Some applications are proposed, in particular the ability for small clusters (animals with one, two or three bonds) to present a singular response for well identified frequencies of the incident electromagnetic field.

Año de publicación:

2000

Keywords:

• 66.30.Dn Theory of diffusion and ionic conduction in solids
• 61.43.Gt Powders, porous materials
• 66.10.Ed Ionic conduction

Fuente:

scopus