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Fourier transforms method for measuring thermal lens induced in diluted liquid samples

Abstract:

Drawing on interferometry and Fourier analysis, this paper describes the use of a two-beam thermal lens technique for measuring thermo-optical properties in optical materials. The procedure consists of yield interference patterns deformed by a localized photothermal effect. The photothermal phase shift is locally induced by the pump beam focused on a tested sample located on an on-axis probe beam, which is the first arm of a Mach-Zehnder interferometer. The plane where the effect is localized is imaged onto a CCD camera. Then two interferograms are recorded: one without effect and the other one with the induced photothermal phase. Fourier analysis performed on these interferograms allow us to plot the thermal lens map and, therefore, to estimate thermo-optic constant of Malachite Green in water solution. The method is applied to measure low linear absorptions of a diluted sample of Rhodamine B in water solution at 633 nm, showing that the proposed technique allows to measure photothermal phase shift as low as 3.1 mrad at 8 mW of input power in diluted materials. © 2007 Elsevier B.V. All rights reserved.