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Reduction of electron-phonon coupling in warm dense iron

Abstract:

The electron-ion relaxation dynamics in warm dense iron were investigated by time-resolved x-ray absorption near-edge spectroscopy (XANES). A novel analysis, combining ab initio density functional theory (DFT) and two temperature model (TTM) simulations, was developed to calculate the x-ray absorption spectra as a function of delay time. Here we present experimental evidence of changes at the XAS L3 edge of iron that are consistent with the reduction of the electron-phonon coupling under warm dense matter conditions. The experimental results are in agreement with the model that takes both the electron (Te) and the ion temperature (Ti) dependence of the thermophysical properties into consideration, while models where either constant electron-phonon coupling factor (G) or only Te-dependent G are used do not agree with the observed relaxation dynamics of iron.