Simultaneous stochastic elects of the solvent and the electromagnetic field on the absorptive and dispersive process in the four wave mixing signal

Abstract:

We calculate the non linear absorptive and dispersive properties in four wave mixing (FWM) signal for a homogeneously broadened molecular two level system with dipole permanent moments interacting with two classical electromagnetic field, using ω1=ω2, considering two sources of noise, the collective effect of the thermal bath, that is modeled as a random Bohr frequency and the effect of the electromagnetic field random amplitude. This assumptions transforms the optical Bloch equations (OBE) to a system of multiplicative stochastic differential equations whose solution is found though an systematic treatment of cumulant expansion which lead directly to reduce OBE. © 2001 SPIE · 0277-786X/01/$15.00.

Año de publicación:

2001

Keywords:

• Two-level system
• stochastic
• FWM

Fuente:

scopus